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I have a closet door that is 81 inches high and 49 inches across
(these measurements are without the jam that is 3/4" thick). With the
jam, the total length across is only 47.5 inches and the standard door
in Home Depot is 24" across (or 48" with 2 doors). Does anyone have
an easy solution?

If I understand what you are trying to do and the doors are going to be
painted. Why not get a couple of 1.5" x 3/8" x 82" strips and glue them to
the side of each door. I think this would be easier than shifting the frame
and the mess will be outside.